Solution:

Answer: $\sqrt{10}$

We claim that the points the ant visits lie on a circle of radius $\frac{\sqrt{10}}{2}$. We show this by saying that the ant stays a constant distance $\frac{\sqrt{10}}{2}$ from the point $\left(\frac{1}{2}, \frac{3}{2}\right)$.

Suppose the ant moves on a plane $P$. Consider a transformation of the plane $P'$ such that after the first move, the ant is at the origin of $P'$ and facing in the direction of the $x'$ axis (on $P'$). The transformation to get from $P$ to $P'$ can be gotten by rotating $P$ about the origin counterclockwise through an angle $\sin^{-1}\left(\frac{3}{5}\right)$ and then translating it 1 unit to the right. Observe that the point $\left(\frac{1}{2}, \frac{3}{2}\right)$ is fixed under this transformation, which can be shown through the expression $\left(\frac{1}{2}+\frac{3}{2} i\right)\left(\frac{4}{5}+\frac{3}{5} i\right)+1=\frac{1}{2}+\frac{3}{2} i$. It follows that at every point the ant stops, it will always be the same distance from $\left(\frac{1}{2}, \frac{3}{2}\right)$. Since it starts at $(0,0)$, this fixed distance is $\frac{\sqrt{10}}{2}$.

Since $\sin^{-1}\left(\frac{3}{5}\right)$ is not a rational multiple of $\pi$, the points the ant stops at form a dense subset of the circle in question. As a result, the least upper bound on the distance between the ant and the origin is the diameter of the circle, which is $\sqrt{10}$.